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Since 1976 the National Coalition to Abolish the Death Penalty has been working to educate the public about the failings and inconsistencies of capital punishment in the United States. Founded after the Gregg v. Georgia Supreme Court decision in 1976, the NCADP has emerged as one of the more influential national anti-death penalty organizations. The collection contains the group's internal case files, administrative material, publications, petitions, photographic materials, video tapes, and audio cassettes.

The M. Watt Espy papers chronicle the extensive research efforts that led to the creation of the Capital Punishment Research Project and the database known as the Espy File. Espy spent three decades gathering and indexing documentation of legal executions in the United States. His papers contain both primary and secondary sources used to catalog thousands of instances of capital punishment in the United States and its territories since the 1600s. The collection includes material from corrections records, newspapers, county histories, legal proceedings, and books. In addition to the records pertaining specifically to the death penalty, there is also a selection of magazines collected by Espy that cover true crime stories as well as life in the American Old West.

Michael A. Mello (1957-2008) was an internationally recognized authority on the death penalty and capital punishment issues. He was a lawyer, professor, and author. Michael Mello served as counsel or informal advisor to many significant cases, including Joseph Robert Crazy Joe Spaziano, Theodore Kaczynski, Theodore Bundy, Rolando Cruz, Alvin Ford, Stephen Todd Booker, and Robert Straight.

Hugo A. Bedau (Ph.D., Harvard, 1961) was a commentator, scholar, and activist for the abolition of capital punishment. He was a prominent spokesperson in the abolitionist movement and well-known for his scholarship and writing concerning the death penalty and the challenge to separate logical arguments from moral arguments.

The Capital Jury Project (CJP) was started in 1991 under the direction of principal investigation, William J. Bowers. The project was funded by an NSF grant to conduct surveys of juror who participated in capital trials. There are three phases to the project.

Bill Pelke is a leader in the national death penalty abolition movement. This collection documents Bill Pelke's involvement with Journey of Hope...from Violence to Healing, Murder Victims' Families for Reconciliation (MVFR), National Coalition to Abolish the Death Penalty (NCADP), Amnesty International, and other organizations committed to ending capital punishment in the United States.

The Bill Babbitt Collection documents nearly ten years of legal efforts to spare Manny Babbitt's life from execution, and two decades of advocacy activities to try to abolish the death penalty.