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The series contains newspaper and magazine articles and interviews relating to Gould's SUNY chancellorship, his involvement on the Commission on Non-Traditional Study, and a 1980 interview covering his educational career. Also included is a folder on the activities of his wife, Laura, and their son's marriage. It also contains a large amount of photographs, both personal and professional in nature. Gould's naval orders and assignments can also be found in this series.

The Samuel B. Gould Papers document his personal life as well as his many professional positions in education, including his tenure as chancellor of the State University of New York.