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The correspondence in this subseries is a mix of letters received by Schaefer as well as carbon copies of letters sent by him or his secretary, Alice Klopfer. The archivist believes that the filing system used in this subseries was created by Ms. Klopfer and has been preserved accordingly. Most folders are titled by the name of the person or company for whom Schaefer was consulting, but there are also files titled simply by letter of the alphabet—these contain correspondence from sources that were not numerous enough to warrant their own folders, and are identified within each folder by subject.

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The documents in this subseries are arranged by name of the organization, institution, or person with whom Schaefer was consulting, followed by a brief indication of the topic(s) within. Schaefer consulted for a wide variety of places, including Boeing; Philip Morris; Arthur D. Little, Inc.; the University of Nevada; Rensselaer Polytechnic Institute and many more. Files include a variety of items such as meeting minutes and reports from organizations Schaefer was working with, company brochures and newsletters, itineraries and vouchers from Schaefer's extensive travels, contract agreements, and correspondence that was not already filed with the letters in subseries #1.

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In addition to serving on the Education Committee of the American Meteorological Society, Schaefer also served on the general council of the AMS. This subseries features documents on the AMS educational films project, correspondence, a few AMS bulletins, and some programs from annual AMS meetings. Although the files do not directly relate to the founding of the Loomis School/NSI, the AMS was responsible for the founding of the Atmospheric Sciences Program at the Loomis School in 1959, and the documentation of educational programs found in this subseries foreshadows the creation of those summer sessions.

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As director of the Loomis School activities, and ultimately as director of research at the Atmospheric Sciences Research Center at the State University of New York, Albany, Schaefer kept records pertaining to the operation of the program. There are many correspondence files; some are between Schaefer and colleagues while others are between Schaefer and the students from the summer program. Numerous students kept in touch with Schaefer well beyond the years that they participated in the Atmospheric Sciences Program, and many of them became successful professionals in their own right.

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Schaefer retained many notebooks kept by the students who participated in the Atmospheric Sciences Program, as well as some of their final papers that detail the projects they worked on for eight weeks. Encouraged by Schaefer to do self-directed experiments, the students kept logs of observations and measurements to aid them in their final reports to staff and peers. A few also sketched illustrations to accompany their notes. Some of the papers in this subseries are final reports of the students' experiments while others are thoughts and reflections on the experience as a whole.