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In addition to traditional photos, the photographs subseries also contains negatives and photo slides. Topics include the environment, chemistry, electrostatics, ice and snow, and world travel. While some of the images in this subseries are directly related to Schaefer's professional work, others are likely derived from extracurricular activities he engaged in while taking photographs for business purposes. Schaefer never did like to let an opportunity go by to explore things that were of interest to him. Some topics, like the Yellowstone Field Expedition, exist as their own subseries elsewhere. In the interests of preserving original order, however, those images were not pulled from this subseries.

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This subseries includes files documenting Vincent Schaefer's varied environmental and outdoor activities that are not associated with a particular organization, such as the Huyck Preserve or Mohonk, or a specific legal effort like the fight to preserve the Great Flats Aquifer. Materials include maps, correspondence, photographs, draft manuscripts, and news clippings. Of interest are folders devoted to the Mohawk Valley Hiking Club, which Schaefer helped found, and his vision for the Long Path, which he saw as a trail for hikers stretching from northern New Jersey through the Adirondacks passing landmarks along the way. Schaefer published articles in this subseries as an individual who loved, studied and appreciated nature, and not as a scientist for General Electric, Munitalp, or the ASRC. Therefore articles in this series span his lifetime. Researchers should note his "Five Rivers Rambles" ongoing series for the Knickerbocker News, written during the early 1970s. In his column, Schaefer explored timely topics, such as air pollution, but also area locations of natural beauty and wonder, including Gore Mountain, the Helderbergs, and Pine Plains.

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The photographs in this subseries date from Schaefer's teenage years all the way through his retirement after he left the Atmospheric Sciences Research Center. Having a love and deep respect for the outdoors from a young age, Schaefer participated in organized activities like the Mohawk Valley Hiking Club, but he also incorporated spontaneous outdoor adventures into his busy schedule whenever he could. Sometimes this meant a day or afternoon exploring areas in and around the Capital Region; other times it meant taking time to explore while he was away on business. His work for General Electric, Munitalp, and the State University at Albany/ASRC (not to mention his extensive consulting) offered ample opportunities to venture into mountain ranges, deserts, plains, valleys, and forests to pursue environmental studies that were of interest to him.