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Schaefer's connection with the University at Albany began in 1959 when the school was still known as the New York State Teachers College, located in downtown Albany. When Schaefer began the highly successful Atmospheric Physics Program via the Loomis School in Connecticut, he attracted the attention of Dean Oscar Lanford and President Evan Collins of the New York State Teachers College. They asked Schaefer to come teach at their Albany school, and within his first year as a faculty member, the idea for the Atmospheric Sciences Research Center (ASRC) was born. Officially established in February 1961, it was originally located in the old General Electric hangar at Schenectady Airport. Although the former New York State Teachers College expanded to the current uptown Albany campus in the mid-1960s, officially becoming the University at Albany, State University of New York, the ASRC remained centered in Schenectady at that time. Meanwhile, the Atmospheric Physics Program that began at the Loomis School shifted to Albany to be under the sponsorship of the ASRC, where it became the Natural Sciences Institute (NSI). However, since the program's roots were not originally with the ASRC and University at Albany, those records comprise their own series within this collection (Series #5).

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This subseries includes reports and publications by Schaefer, his colleagues at the ASRC, and colleagues from other institutions who worked closely with Schaefer and occasionally collaborated with the ASRC. Names from the latter group will sound familiar from Schaefer's consulting materials, such as Wendell Mordy and Paul MacCready. Topics range from annual ASRC reports, to solar energy work, to particle studies and more. Some documents are official reprints of articles while others are handwritten manuscripts or typescripts.

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The subject files feature a variety of materials that supplement Schaefer's Munitalp research documents, such as ephemera from some of his many travels, conference brochures, and weather research activities of groups not affiliated with Munitalp. This subseries also includes administrative files such as personnel information, grant writing endeavors, and budgeting, which are reflections of Schaefer's role as director of research. There are also photographs of Schaefer and colleagues, non-Skyfire research projects, travels in and out of the United States, and more generic subjects such as research equipment.