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This series contains a variety of materials from Vincent Schaefer's personal life, some of it autobiographical. Subseries one features his unpublished memoir, Twenty Years at Langmuir University, but also family photographs, an extensive personal log, and awards. The series also documents his passions for hiking, Scouting, skiing, geology, artwork, Dutch Barns, local history and archeology.

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The Vincent Schaefer personal subseries comprises material spanning his life and career and pertains only to personal interests outside the realms of his atmospheric and prescribed research ventures. This subseries contains his schedules and itineraries, along with Schaefer's personal logs from 1947 through 1993. Along with Schaefer's own autobiography Twenty Years at Langmuir University there are timelines, resumes, and lists of works published, all created by Schaefer.